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The multidentate 4-aminotriazole-bridged organic ligand 4-amino-3,5-bis(4,3′-bipyridyl-5′-yl)-4H-1,2,4-triazole has been prepared and used to synthesize two CoII coordination polymers, under solvothermal conditions, both featuring two-dimensional networks. The aminotriazole functions as a bidentate cis-conformation ligand linking the CoII ions in one complex, while it functions as a tridentate trans-conformation linker binding CoII ions in the other complex.