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A novel family of four 1-bromo-2,6-bis{[(λ5-phosphanylidene)imino]methyl}benzene ligands has been synthesized and each ligand has been complexed with nickel(II). The phosphinimine substituents incrementally change from all-phenyl to all-cyclohexyl across this family and these ligands represent a useful opportunity to investigate the impact of changing sterics on complex structure and reactivity.