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Two Fe3(CO)8([mu]3-S)2 clusters with terminal N-heterocyclic carbenes have been synthesized. Of the eight carbonyl ligands, one deviates significantly from linearity. In one cluster, N-H...S and C-H...O hydrogen bonds combine the mol­ecules into [101] sheets, while in the other cluster, N-H...S and C-H...O inter­actions link the mol­ecules into [111] chains.
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