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In the crystal structure of the title compound, [Zn(NCS)2(C6H8N2)2], the Zn atom and both iso­thio­cyanate groups lie on a crystallographic mirror plane. The Zn atom is in a distorted tetrahedral geometry. The crystal structure is stabilized by N—H...S hydrogen bonds and weak π–π interactions.

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In the centrosymmetric title compound, [Cd(NCS)2(C6H8N2)4], the CdII atom is in a distorted octa­hedral environment. The crystal structure is stabilized by N—H...S hydrogen bonds and weak N—H...π and C—H...π inter­actions.
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