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The centrosymmetric main mol­ecule of the title compound, [Fe2(C5H5)2(C16H16N4O2S2)]·2CHCl3, contains two linked ferrocene groups and possesses intramolecular N—H...O hydrogen bonds with an S(6) graph-set motif. Two CHCl3 solvent mol­ecules interact with the main species by way of C—H...O interactions. Intermolecular N—H...S and C—H...S interactions link the mol­ecules into one-dimensional chains with an R21(7) motif.
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